Dimensionality control of electronic phase transitions in nickel-oxide superlattices.
نویسندگان
چکیده
The competition between collective quantum phases in materials with strongly correlated electrons depends sensitively on the dimensionality of the electron system, which is difficult to control by standard solid-state chemistry. We have fabricated superlattices of the paramagnetic metal lanthanum nickelate (LaNiO(3)) and the wide-gap insulator lanthanum aluminate (LaAlO(3)) with atomically precise layer sequences. We used optical ellipsometry and low-energy muon spin rotation to show that superlattices with LaNiO(3) as thin as two unit cells undergo a sequence of collective metal-insulator and antiferromagnetic transitions as a function of decreasing temperature, whereas samples with thicker LaNiO(3) layers remain metallic and paramagnetic at all temperatures. Metal-oxide superlattices thus allow control of the dimensionality and collective phase behavior of correlated-electron systems.
منابع مشابه
Oxide interfaces: Instrumental insights.
S ir Arthur Stanley Eddington said, " We used to think that if we knew one, we knew two, because one and one are two. We are finding that we must learn a great deal more about 'and'. " Combining multiple materials with desirable properties is an oft-pursued route to achieve artificial composite materials with functionalities superior to any of their parts. When the dimensions at which the const...
متن کاملDimensionality Control of d-orbital Occupation in Oxide Superlattices
Manipulating the orbital state in a strongly correlated electron system is of fundamental and technological importance for exploring and developing novel electronic phases. Here, we report an unambiguous demonstration of orbital occupancy control between t2g and eg multiplets in quasi-two-dimensional transition metal oxide superlattices (SLs) composed of a Mott insulator LaCoO3 and a band insul...
متن کاملتشدید شکل فشباخ برای جفت شدگی Tc بالا در ابرشبکههای نوارهای کوانتمی و چاههای کوانتمی
The Feshbach shape resonances in the interband pairing in superconducting superlattices of quantum wells or quantum stripes is shown to provide the mechanism for high Tc superconductivity. This mechanism provides the Tc amplification driven by the architecture of material: superlattices of quantum wells (intercalated graphite or diborides) and superlattices of quantum stripes (doped high Tc c...
متن کاملInterplay between Cation and Charge Ordering in La1/3Sr2/3FeO3 Superlattices
DOI: 10.1002/aelm.201500372 superlattices, in particular the (LaMnO3)m/ (SrMnO3)n system, has yielded important insights into the relationships between charge transfer, electronic structure, cation disorder, and magnetic ordering.[11–15] Ferroelectric superlattices have also received considerable attention,[16–18] with short-period superlattices emerging as a platform in which to realize improp...
متن کاملStrain-controlled Insulator-Metal Transition in YTiO3/SrTiO3 Superlattices: A First-Principles Study
The structural, magnetic, and electronic properties of (STO)4/(YTO)2 superlattice consisting of Mott insulator YTiO3 (YTO) and band insulator SrTiO3 (STO) under strain are investigated by the density-functional-theory plus U method. It is found that an insulator-metal transition occurs when a compressive strain of 0.2% is applied. The structural analyses reveal that the presence of metallic sta...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید
ثبت ناماگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید
ورودعنوان ژورنال:
- Science
دوره 332 6032 شماره
صفحات -
تاریخ انتشار 2011